The Dark Crow Smiles is used in the anime and is sung by Lotus Juice in English, but the chorus is sung in Latin. It's a Catholic song called "Agnus Dei" which means Lamb of God.
It's track number 10 on disc 1 of Kuroshitsuji Sound Complete Black Box. And it can be heard in track number 14 on disc 2 as a remix.
This is made for season 1.
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Kuroshitsuji/ Black Butler songs
Художественная прозаHere are (probably) all Kuroshitsuji/ Black Butler openings, endings, character songs, OSTs and CDs. There will also be the character songs that are made as a headcanon by most of the fandom. Btw, sorry if there are English grammar/ spelling mistak...
